Vibrational characterization of catalytic intermediates in a dual cryogenic ion trap spectrometer
Duffy, Erin M.
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https://hdl.handle.net/2142/91460
Description
Title
Vibrational characterization of catalytic intermediates in a dual cryogenic ion trap spectrometer
Author(s)
Duffy, Erin M.
Contributor(s)
Garand, Etienne
Marsh, Brett
Voss, Jonathan
Issue Date
2016-06-22
Keyword(s)
Spectroscopy in Traps
Abstract
Decades of research on water oxidation catalysis has yielded much progress in making water splitting a viable option for alternative energy. However, precise molecular-level understanding of the catalytic mechanism remains elusive due to the difficulty of studying reaction intermediates by traditional methods. In this talk, vibrational characterization of a ruthenium water oxidation catalyst and catalytic intermediates will be presented. In particular, infrared spectra acquired using a recently developed approach that employs two cryogenic ion traps, which enable the isolation of the chemical species discussed here, will be the focus of this talk.
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