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https://hdl.handle.net/2142/84476
Description
Title
Chemistry of Carbon Sulfides
Author(s)
Breitzer, Jonathan Gabriel
Issue Date
2000
Doctoral Committee Chair(s)
Rauchfuss, Thomas B.
Department of Study
Chemistry
Discipline
Chemistry
Degree Granting Institution
University of Illinois at Urbana-Champaign
Degree Name
Ph.D.
Degree Level
Dissertation
Keyword(s)
Chemistry, Inorganic
Language
eng
Abstract
The third-order nonlinear optical susceptibilities of carbon sulfides, along with other sulfur-rich metal complexes, were measured using the z-scan technique with a 35 ps pulsed laser at 527.5 nm. The measurements were done in solution, which was continuously pumped through the sample cuvette to avoid heating. The susceptibilities of the molecules in solution was determined by subtracting the susceptibility of the solvent from that of the solution. The highest susceptibilities were found to be for C6S8O 2 and (Me4N)4[Zn10(SPh)16].
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