Atom-by-Atom Substitution of Transition Metals in Gallium Arsenide and Visualization of Hole-Mediated Interactions
Kitchen, Dale Spencer
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https://hdl.handle.net/2142/80542
Description
Title
Atom-by-Atom Substitution of Transition Metals in Gallium Arsenide and Visualization of Hole-Mediated Interactions
Author(s)
Kitchen, Dale Spencer
Issue Date
2006
Doctoral Committee Chair(s)
Yazdani, Ali
Department of Study
Physics
Discipline
Physics
Degree Granting Institution
University of Illinois at Urbana-Champaign
Degree Name
Ph.D.
Degree Level
Dissertation
Keyword(s)
Physics, Condensed Matter
Language
eng
Abstract
We also present the first controlled atomic scale study of the interactions between isolated Mn impurities mediated by electronic states in GaAs. High-resolution STM measurements provide visualization of the GaAs electronic states that participate in Mn-Mn interactions. We quantify the interaction strengths between Mn pairs as a function of relative position and orientation. Our experimental findings, which can be explained using tight-binding model calculations, reveal a strong dependence of ferromagnetic interaction on crystallographic orientation. This anisotropic interaction can potentially be exploited by growing oriented Ga1-xMnxAs structures to enhance the ferromagnetic transition temperature beyond that achieved in randomly doped samples.
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