Luminescence characteristics of single and multiple aluminum gallium arsenide-gallium arsenide quantum-well heterostructure lasers
Kolbas, Robert Michael
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https://hdl.handle.net/2142/25548
Description
Title
Luminescence characteristics of single and multiple aluminum gallium arsenide-gallium arsenide quantum-well heterostructure lasers
Author(s)
Kolbas, Robert Michael
Issue Date
1979
Doctoral Committee Chair(s)
Holonyak, Nick, Jr.
Department of Study
Physics
Discipline
Physics
Degree Name
Ph.D.
Degree Level
Dissertation
Keyword(s)
luminescence
aluminum gallium arsenide-gallium arsenide
quantum-well heterostructure lasers
metalorganic chemical vapor deposition
Language
en
Abstract
The luminescence properties of single and multiple A1x Gal-x As-GaAs
quantum-well heterostructure lasers grown by meta10rganic chemical vapor deposition (MO-CVD) are shown to differ markedly from those of conventional double heterojunctions because of the two-dimensional nature of the active region. The experimental characteristics of quantum-well recombination radiation are presented and are explained in terms of the properties of quantized carrier motion. Photopumped single quantum-well A1x Gal-x As-GaAs-A1x Gal-x As (x-O. 6, Lz=well width -200 A) heterostructures are shown to operate (77°K) on
z confined-particle transitions from the infrared to the red (6885 A, ~A-1300 A, Delta E=hw-E -293 meV). Two fundamental limitations of single
quantum-well A1GaAs-GaAs heterostructures are identified. The first is
concerned with the highest energy emission obtainable, and is related to
the position of the L indirect minima in GaAs. The location of the first indirect conduction band minima (L minima) is determined by a luminescence
(emission) technique and is found to be -294 meV above the r band edge at 4.3°K. The second limitation involves the loss of luminescence efficiency as the well thickness Lz approaches the carrier scattering path length
lp, where lp -63 A is the electron scattering length with longitudinal
optical (LO) phonons. In addition, the band discontinuities between AIGaAs
and GaAs are measured by a technique based on the recombination of free electrons in the AIGaAs with bound 'holes in the GaAs well.
The carrier collection problem associated with a small single well can be overcome by coupling several thin GaAs quantum layers via thin A1GaAs barriers so as to form a composite active region considerably larger than the scattering length t. These multiple-well structures operate as
p lasers continuously at room temperature (CW 3000 K) at energies as high as
145 meV above the GaAs r band edge (hw-Eg -0-145 meV). In addition, data
showing CW 3000 K laser operation at photoexcitation threshold levels 2 2
(900W/cm2 , Jth ~375A/cm2 ) comparable to better LPE double heterojunctions
and much lower than all previous single or multiple quantum-well heterostructures are presented.
The origin of quantum-well recombination radiation below the lowest allowed confined-particle transition is discussed and is identified as
phonon-assisted recombination. Phonon-sideband laser data (4.3-3000 K)
are presented showing emission at 36, 72, and 108 meV (integer multiples of E-36 meV) below the lowest confined-particle transition. Phonon
involvement is also shown to occur throughout the entire direct-gap range of these quantum-well heterostructures. In addition, data are presented indicating that the electron-phonon interaction is enhanced as the number of coupled quantum wells in the active region is increased. A qualitative analysis and discussion of the observed electron-phonon interaction is presented. The origin of this interaction is related to the two-dimensional nature of these structures, and the analysis suggests that stimulated phonon emission is possible in the quantum-well heterostructures of this work.
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