Temperature-dependent Water Uptake Behavior Of Clusters Relevant To New Particle Formation
Kreinbihl, John J.
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5431.pdf
FE03_5431.pdf
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https://hdl.handle.net/2142/111241
Description
Title
Temperature-dependent Water Uptake Behavior Of Clusters Relevant To New Particle Formation
Author(s)
Kreinbihl, John J.
Contributor(s)
Johnson, Christopher J.
Frederiks, Nicoline C.
Issue Date
2021-06-25
Keyword(s)
Atmospheric science
Date of Ingest
2021-09-24T21:09:20Z
2022-01-21T16:09:42Z
Abstract
New particle formation is a process in which trace vapors in the atmosphere cluster and grow into larger particles. Recently, we have employed a multi-trap gas-phase ion preparation technique and cryogenic ion vibrational predissociation (CIVP) spectroscopy to identify common structural motifs for the uptake of water into cationic clusters relevant to NPF. Here we further extend this exploration using a multi-trap gas phase variable temperature mass spectrometry (VTMS) technique in which we probe the water uptake of clusters as a function of temperature to determine the associated thermodynamic parameters. We then seek to correlate these water uptake parameters to structural motifs present in the dry clusters.
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5431.pdf
FE03_5431.pdf
