This talk will provide an introduction to this mini-symposium, which
features advances in high-harmonic generation and the spectroscopy it enables.
This strong-field process is a sensitive probe of small-molecule electronic
structure, as the spectrum of the extreme ultraviolet (XUV) photons produced
by the ionization-recollision process measures the shape and energy of the
molecular orbitals. Furthermore, the XUV pulse can be used as an
element-specific probe of electron dynamics in molecules and materials
at femtosecond to attosecond timescales.
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